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科自福到来岛的加州探测性硫研人员在放射
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简介PNAS:科研人员在加州探测到来自福岛的放射性硫 2011-08-16 09:35 · diana ...
PNAS:科研人员在加州探测到来自福岛的科研放射性硫
2011-08-16 09:35 · diana科研人员在加利福尼亚州的La Jolla发现了来自福岛第一核电站的放射性硫。这组作者报告说,加州
生物探索推荐英文论文摘要:
Evidence of neutron leakage at the Fukushima nuclear plant from measurements of radioactive 35S in California
Abstract
A recent earth*** and 探测the subsequent tsunami have extensively damaged the Fukushima nuclear power plant, releasing harmful radiation into the environment. Despite the obvious implication for human health and the surrounding ecology, there are no quantitative estimates of the neutron flux leakage during the weeks following the earth***. Here, using measurements of radioactive 35S contained in sulfate aerosols and SO2 gas at a coastal site in La Jolla, California, we show that nearly 4 × 1011 neutrons per m2 leaked at the Fukushima nuclear power plant before March 20, 2011. A significantly higher 35SO4-2activity as measured on March 28 is in accord with neutrons escaping the reactor core and being absorbed by the coolant seawater 35Cl to produce 35S by a (n, p) reaction. Once produced, 35S oxidizes to 35SO2and 35SO4-2and was then transported to Southern California due to the presence of strong prevailing westerly winds at this time. Based on a moving box model, we show that the observed activity enhancement in 35SO4-2is compatible with long-range transport of the radiation plume from Fukushima. Our model predicts that 35SO4-2, the concentration in the marine boundary layer at Fukushima, was approximately 2 × 105 atoms per m3, which is approximately 365 times above expected natural concentrations. These measurements and model calculations imply that approximately 0.7% of the total radioactive sulfate present at the marine boundary layer at Fukushima reached Southern California as a result of the trans-Pacific transport.
大气中的到自的放放射性硫离子和二氧化硫气体的浓度在2011年3月28日最高。这些发现表明了可以使用硫同位素作为空气传播的福岛化学物质的转变和长距离输运的一个标记物。科研人员在加利福尼亚州的射性La Jolla发现了来自福岛第一核电站的放射性硫。通过一个建模分析,科研与自从2009年2月起该地区记录到的加州背景水平相比,这组作者说,探测Mark H. Thiemens及其同事从2011年3月9日到4月1日在Scripps海洋学研究所位于La Jolla的栈桥测量了核爆炸产生的放射性硫在含有矿物质的海水以及空气中的含量。这组作者估计,
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